Tracks
| # | Title | Sung by | |
|---|---|---|---|
| 1 | (Theme From) The Man From U.N.C.L.E. | Jerry Goldsmith | 2:04 |
| 2 | Meet Mr. Solo | Jerry Goldsmith | 2:29 |
| 3 | A Martini Built for Two | Morton Stevens | 2:27 |
| 4 | Wild Bike | Morton Stevens | 2:34 |
| 5 | Solo on a Raft | Walter Scharf | 1:54 |
| 6 | Fiddlesticks | Lalo Schifrin | 2:14 |
| 7 | The Man From Thrush | Lalo Schifrin | 2:10 |
| 8 | Illya | Lalo Schifrin | 2:09 |
| 9 | The Invaders | Jerry Goldsmith | 2:30 |
| 10 | Solo's Samba | Walter Scharf | 2:29 |
| 11 | Bye, Bye Jill | Morton Stevens | 2:12 |
| 12 | Watch Out | Walter Scharf | 2:40 |
| 13 | Sandals Only | Gerald Fried | 2:36 |
| 14 | Solo Busanova | Robert Drasnin | 2:11 |
| 15 | Off and Running | Robert Drasnin | 2:30 |
| 16 | Boo-Bam-Boo, Baby | Gerald Fried | 1:53 |
| 17 | Slink | Gerald Fried | 2:13 |
| 18 | Run Spy Run | Gerald Fried | 2:16 |
| 19 | Jungle Beat | Gerald Fried | 2:01 |
| 20 | The Wiggely Pig Walk | Gerald Fried | 2:09 |
| 21 | Lament for a Trapped Spy | Gerald Fried | 2:23 |
| 22 | There They Go | Robert Drasnin | 2:11 |
| 23 | Jo Jo's Torch Thing | Robert Drasnin | 2:15 |
| 24 | Dance of the Flaming Swords | Gerald Fried | 2:38 |
Source: MusicBrainz release group fb031686-8035-3d91-b3dc-201ca978634c (CC0). Cover: Cover Art Archive.