| 1.1 | All or Nothing at All | Frank Sinatra | 2:58 |
| 1.2 | From the Bottom of My Heart | Frank Sinatra | 3:09 |
| 1.3 | If I Didn’t Care | Frank Sinatra | 3:31 |
| 1.4 | Moon Love | Frank Sinatra | 2:59 |
| 1.5 | East of the Sun (and West of the Moon) | Frank Sinatra, The Sentimentalists | 3:20 |
| 1.6 | I’ll Be Seeing You | Frank Sinatra | 3:04 |
| 1.7 | Say It | Frank Sinatra | 3:25 |
| 1.8 | Blue Skies | Frank Sinatra, [unknown] | 3:17 |
| 1.9 | I’ll Never Smile Again | Frank Sinatra | 3:12 |
| 1.10 | Fools Rush In (Where Angels Fear to Tread) | Frank Sinatra with Tommy Dorsey and His Orchestra | 3:14 |
| 1.11 | This Love of Mine | Frank Sinatra | 3:44 |
| 1.12 | Oh! Look at Me Now | Frank Sinatra with Connie Haines, The Pied Pipers & Tommy Dorsey and His Orchestra | 3:17 |
| 1.13 | Just as Though You Were Here | Frank Sinatra with The Pied Pipers & Tommy Dorsey and His Orchestra | 3:14 |
| 1.14 | How About You? | Frank Sinatra with Tommy Dorsey and His Orchestra | 2:55 |
| 1.15 | Imagination | Frank Sinatra | 3:15 |
| 1.16 | Frenesi | Frank Sinatra, Jo Stafford, The Pied Pipers, Clark Yocum, Chuck Lowry, John Huddleston | 3:38 |
| 1.17 | Blue Moon | Frank Sinatra | 3:41 |
| 1.18 | Be Careful, It’s My Heart | Frank Sinatra | 2:47 |
| 1.19 | The Song Is You | Frank Sinatra | 3:22 |
| 1.20 | Night and Day | Frank Sinatra with Axel Stordahl and His Orchestra | 3:03 |
| 2.1 | No Love, No Nothin’ | Frank Sinatra | 2:55 |
| 2.2 | Saturday Night (Is the Loneliest Night of the Week) | Frank Sinatra | 2:45 |
| 2.3 | Oh! What It Seemed to Be | Frank Sinatra | 2:52 |
| 2.4 | You’ll Never Know | Frank Sinatra | 3:24 |
| 2.5 | I’ve Got a Crush on You | Frank Sinatra | 3:19 |
| 2.6 | The Brooklyn Bridge | Frank Sinatra | 2:38 |
| 2.7 | Five Minutes More | Frank Sinatra | 2:46 |
| 2.8 | (It Seems to Me) I’ve Heard That Song Before | Frank Sinatra | 3:03 |
| 2.9 | The Trolley Song | Frank Sinatra | 3:07 |
| 2.10 | Time After Time | Frank Sinatra | 3:11 |
| 2.11 | Dream (When You’re Feeling Blue) | Frank Sinatra with the Ken Lane Singers | 3:03 |
| 2.12 | I Fall in Love Too Easily | Frank Sinatra | 3:17 |
| 2.13 | She’s Funny That Way | Frank Sinatra | 3:22 |
| 2.14 | It’s Been a Long, Long Time | Frank Sinatra, June Hutton, The Pied Pipers, Hal Hopper, Clark Yocum, Chuck Lowry | 3:01 |
| 2.15 | Dancing in the Dark | Frank Sinatra, The Vimms Chorale | 4:04 |
| 2.16 | I’ve Got You Under My Skin / Easy to Love | Frank Sinatra, The Vimms Chorale | 4:06 |
| 2.17 | Nancy (With the Laughing Face) | Frank Sinatra | 3:14 |
| 2.18 | Lover Come Back to Me | Frank Sinatra, Bobby Tucker, Bobby Trucker Singers | 3:58 |
| 2.19 | Put Your Dreams Away | Frank Sinatra | 3:10 |
| 2.20 | Again | Frank Sinatra with Johnny Green and His Orchestra | 2:10 |
| 3.1 | All of Me | Frank Sinatra | 2:42 |
| 3.2 | Sweet Lorraine | Frank Sinatra with Metronome All Stars | 3:10 |
| 3.3 | Body and Soul | Frank Sinatra feat. Bobby Hackett | 3:20 |
| 3.4 | All the Things You Are | Frank Sinatra, Ken Lane, Ken Lane Singers | 3:04 |
| 3.5 | Embraceable You | Frank Sinatra | 2:54 |
| 3.6 | These Foolish Things (Remind Me of You) | Frank Sinatra | 3:09 |
| 3.7 | Stormy Weather | Frank Sinatra, Ken Lane Singers | 4:16 |
| 3.8 | Begin the Beguine | Frank Sinatra | 3:56 |
| 3.9 | There Will Never Be Another You | Frank Sinatra | 2:15 |
| 3.10 | As Time Goes By | Frank Sinatra | 2:34 |
| 3.11 | The Nearness of You | Frank Sinatra | 2:44 |
| 3.12 | Stella by Starlight | Frank Sinatra, The Pied Pipers | 3:22 |
| 3.13 | I Get a Kick Out of You | Frank Sinatra with The Vimms Chorale | 3:58 |
| 3.14 | That Old Black Magic | Frank Sinatra | 2:34 |
| 3.15 | One for My Baby (and One More for the Road) | Frank Sinatra | 3:06 |
| 3.16 | It Had to Be You | Frank Sinatra | 2:31 |
| 3.17 | What’ll I Do | Frank Sinatra | 3:07 |
| 3.18 | Laura | Frank Sinatra | 3:20 |
| 3.19 | September Song | Frank Sinatra | 3:07 |
| 3.20 | Ol’ Man River | Frank Sinatra | 4:01 |
| 4.1 | The Birth of the Blues | Frank Sinatra | 3:29 |
| 4.2 | April in Paris | Frank Sinatra with The Whippoorwills | 2:45 |
| 4.3 | American Beauty Rose | Frank Sinatra | 2:36 |
| 4.4 | Lover | Frank Sinatra | 2:42 |
| 4.5 | The Continental | Frank Sinatra | 2:33 |
| 4.6 | Should I (Reveal) | Frank Sinatra | 2:25 |
| 4.7 | When You’re Smiling (the Whole World Smiles With You) | Frank Sinatra | 2:32 |
| 4.8 | It All Depends on You | Frank Sinatra | 3:25 |
| 4.9 | Bye Bye Baby | Frank Sinatra | 2:40 |
| 4.10 | I Could Write a Book | Frank Sinatra | 2:44 |
| 4.11 | Autumn in New York | Frank Sinatra | 3:17 |
| 4.12 | If Only She’d Looked My Way | Frank Sinatra | 2:50 |
| 4.13 | Hello Young Lovers | Frank Sinatra | 3:35 |
| 4.14 | We Kiss in a Shadow | Frank Sinatra | 3:38 |
| 4.15 | My Girl | Frank Sinatra | 2:27 |
| 4.16 | Love Me | Frank Sinatra | 3:10 |
| 4.17 | Farewell, Farewell to Love | Frank Sinatra | 2:56 |
| 4.18 | Walking in the Sunshine | Frank Sinatra | 2:43 |
| 4.19 | Why Try to Change Me Now | Frank Sinatra | 2:50 |
| 4.20 | I’m a Fool to Want You | Frank Sinatra | 2:56 |